xu2015
xu2015
xu2015
a r t i c l e i n f o a b s t r a c t
Article history: Pool boiling heat transfer of metal foams with gradient pore densities has been investigated at atmo-
Received 28 October 2014 spheric pressure in saturated deionized water. The gradient foams are made of two foam layers. The foam
Received in revised form 9 February 2015 materials are copper and nickel. Pore densities of foam layers are from 5 PPI to 100 PPI, while the porosity
Accepted 9 February 2015
remains the fixed value of 0.98. A parametric study is performed by varying the foam pore size and
thickness. The effects of alumina nanoparticles and surfactant (SDS) on pool boiling heat transfer of
gradient metal foams are also investigated in the present study. Images of foam fiber deposited by
Keywords:
nanoparticles are captured by SEM. Compared to single-layer foams, gradient metal foams significantly
Pool boiling
Gradient metal foam
enhance pool boiling heat transfer and the enhancement is heavily dependent on foam thickness and
Morphology pore density gradient. The effects of SDS and nanoparticles on pool boiling heat transfer of gradient foams
Nanoparticle are dependent on concentrations.
Surfactant Ó 2015 Elsevier Ltd. All rights reserved.
http://dx.doi.org/10.1016/j.ijheatmasstransfer.2015.02.017
0017-9310/Ó 2015 Elsevier Ltd. All rights reserved.
Z.G. Xu, C.Y. Zhao / International Journal of Heat and Mass Transfer 85 (2015) 824–829 825
gradient metal foams. Nanoparticle, surfactant and foam pore size, 3. Results and discussion
thickness effects have been studied in the present study.
3.1. Morphology effect
2. Experiment and metal foam parameters
Pool boiling curves of gradient nickel foams with the pore den-
The whole experimental facility consists of a heating system, a sity variation from 20 PPI to 5 PPI are shown in Fig. 2(a, b). In the
cooling system and a data acquisition system (Fig. 1). The present study, GF-20 PPI–2 mm & 5 PPI–4 mm-Ni represents a gra-
water/nanofluid in the chamber is heated by the two auxiliary hea- dient nickel foam made of 20 PPI down foam layer with the thick-
ters to its saturation point, and then cooled down to the surround- ness of 2 mm and 5 PPI up foam layer with the thickness of 4 mm,
ing temperature naturally to remove the non-condensable gas SF-20 PPI–2 mm–Ni represents a single-layer nickel foam with the
outside. In the experiment, the two auxiliary heaters are first thickness of 2 mm, and similar specifications are used for other
switched on to keep the working water/nanofluid saturated, then cases. It can be found that, sintering 5 PPI nickel foam on 20 PPI
the main heater is switched on to heat the sample substrate from nickel foam surface remarkably enhances the latter’s pool boiling
the beginning heat flux of 8 103 W m2. The thermocouple sig- heat transfer. The up foam layer with a low pore density provides
nals are collected by the Keithley data acquisition unit when their bigger connected pores more space for escaping bubbles from the
variation is within 0.2 K per 20 min. The above procedure is repeat- lower foam layer surface, increases collision time between bubbles
ed when the heat flux increases by the step of 5 104 to and foam skeleton and prolongs bubble growth period inside
10 104 W m2. The maximum uncertainty of is 8.9% by perform- foams. According to the fiber diameter and surface area density
ing the standard uncertainty analysis. More details of the experi- based on the microstructure model of uniform metal foams [18],
ment can be found in the authors’ previous study [17]. In the total surface area of a gradient metal foam can be calculated as:
present study, foam layers were sintered together by Ag–Cu alloy X
n qffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
sheets in a high-temperature muffle furnace to form gradient met- Stotal V i 4ðp þ p2 Þð1 ei Þ=dpi ð1Þ
al foams (Fig. 1). Foam porosity is fixed as 0.98, and thickness is i¼1
from 6 mm to 20 mm. The foam material is copper and nickel. where n is foam layer number, e is a foam layer porosity. One foam
Single-layer metal foams are considered as the reference samples layer volume V and pore diameter dp can be respectively calculated
for the comparison purpose. Images of deposited nanoparticle lay- as:
ers on foam fibers were captured by SEM (Sirion 200, Instrument
Analysis Center of SJTU). V ¼ 0:025 0:025 d ð2Þ
Fig. 1. Sketch of the experimental facility and gradient metal foams (all dimensions are in mm).
826 Z.G. Xu, C.Y. Zhao / International Journal of Heat and Mass Transfer 85 (2015) 824–829
q(W· m )
-2
i¼1 5
qffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi 6.0x10
4ðp þ p2 Þð1 ei Þ=0:0254 ð4Þ 5
4.0x10
GF-20 PPI-2 mm & 5 PPI-8 mm-Ni
According to Eq. (4), surface area increments by sintering upper GF-20 PPI-4 mm & 5 PPI-8 mm-Ni
5
foam layers 5 PPI–4 mm, 5 PPI–6 mm and 5 PPI–8 mm on the foam 2.0x10 GF-20 PPI-6 mm & 5 PPI-8 mm-Ni
layer 20 PPI–2 mm are 50%, 75% and 100%, respectively. However, SF-5PPI-8 mm-Ni
smooth copper plate
from the result shown in Fig. 2(a), it can be found that surface area 0.0
0 10 20 30
increment has little effect on the pool boiling heat transfer
ΔTsat(K)
enhancement degree. Surface area increment by sintering upper
foam layers 5 PPI–4 mm, 5 PPI–6 mm and 5 PPI–8 mm on the foam (a) upper layer = 8 mm (20 PPI & 5 PPI)
layer 20 PPI–8 mm are 16.67%, 25% and 33.3%, respectively.
Fig. 2(b) indicates that pool boiling heat transfer enhancement 6
1.2x10
degree firstly decreases and then increases with increasing foam
thickness. The maximum pool boiling heat transfer coefficient 6
1.0x10
increment by the nickel foam 5 PPI–8 mm is about 500% at the heat
flux of 5 105 W m2. Surface area increments by sintering the 5
foam layer 5 PPI–8 mm on the foam layers 20 PPI–2 mm, 20 PPI– 8.0x10
4 mm, 20 PPI–6 mm are 100%, 50% and 33.3%. The results shown q(W· m )
-2
5
in Fig. 3(a) indicate that the pool boiling heat transfer enhance- 6.0x10
ment degree increases with increasing 20 PPI foam thickness. 5
According to Eq. (4), surface area increment by sintering the 4.0x10
GF-100 PPI-2 mm & 5 PPI-8 mm-Ni
upper foam layer 5 PPI–8 mm on the foams layers 100 PPI– 5
GF-100 PPI-4 mm & 5 PPI-8 mm-Ni
2.0x10 GF-100 PPI-6 mm & 5 PPI-8 mm-Ni
SF-5 PPI-8 mm-Ni
smooth copper plate
1.2x10
6 0.0
0 10 20 30
ΔTsat(K)
6
1.0x10
(b) upper layer =8 mm (100 PPI & 5 PPI )
5
8.0x10
Fig. 3. Lower foam layer thickness effect.
q(W· m )
-2
5
6.0x10
2 mm,100 PPI–4 mm,100 PPI–6 mm are 20%, 10%, 6.67%, respec-
5
4.0x10 tively, which indicates surface area increment decreases. Pool boil-
GF-20 PPI-2 mm & 5 PPI-4 mm-Ni
GF-20 PPI-2 mm & 5 PPI-6 mm-Ni
ing heat transfer of GF-100 PPI & 5 PPI increases with increasing
5
2.0x10 GF-20 PPI-2 mm & 5 PPI-8 mm-Ni foam thickness, as shown in Fig. 3(b).Compared with the single
SF-20 PPI-2 mm-Ni
smooth copper plate
foam SF-5 PPI–8 mm-Ni, at low heat fluxes, pool boiling heat trans-
0.0 fer performance of GF-100 PPI & 5 PPI is superior because of higher
0 10 20 30
ΔTsat(K)
surface area. 100 PPI nickel foam has many small pores which
providing a large number of nucleation sites during the boiling
(a) lower layer=2 mm(20PPI&5PPI) process. However, bubbles’ number and volume increases with
increasing heat flux, and they suffer more serious resistance from
1.2x10
6 foam skeleton because of the limited space of connected pores.
Therefore, pool boiling heat transfer coefficient of GF-100 PPI &
1.0x10
6 5 PPI is lower than SF-5 PPI–8 mm-Ni when the heat flux is over
7 105 W m2. Compared the results shown in Fig. 3(b) with those
8.0x10
5 shown in Fig. 3(a), it can be found that, sintering a foam with a low
pore density on a foam with a middle pore density far outstrips a
q(W· m )
-2
6.0x10
5 foam with a high pore density.
5
4.0x10 3.2. Nanoparticle effect
GF-20 PPI-6 mm & 5 PPI-4 mm-Ni
5 GF-20 PPI-6 mm & 5 PPI-6 mm-Ni
2.0x10 GF-20 PPI-6 mm & 5 PPI-8 mm-Ni Fig. 4(a–c) indicate that, adding alumina particle into boiling
SF-20 PPI-6 mm-Ni
smooth copper plate
water worsens pool boiling heat transfer of GF-20 PPI–4 mm &
0.0 5 PPI–8 mm-Cu because the thermal conductivity of alumina
0 10 20 30
(26.8 W m1 K1) is far lower than the copper (398 W m1 K1).
ΔTsat(K)
The 100 nm alumina deposition effect on GF-20 PPI–4 mm &
(b) 5 PPI-8 mm-Cu and GF-100 PPI–4 mm & 5 PPI–8 mm-Cu are shown
lower layer = 6 mm(20 PPI & 5 PPI)
in Fig. 5(a) and (b), respectively. Deposited alumina nanoparticles
Fig. 2. Upper foam layer thickness effect. worsen pool boiling heat transfer of the two gradient copper
Z.G. Xu, C.Y. Zhao / International Journal of Heat and Mass Transfer 85 (2015) 824–829 827
,
1.4x10
6
X
n
d¼m Si q ð7Þ
6
1.2x10 i¼1
1.0x10
6
where m is the deposited nanoparticle weight, q is the nanoparticle
5 density.
8.0x10
Alumina nanoparticle weight is weight difference between the
q(W· m )
-2
5
6.0x10 copper foams with and without deposited alumina nanoparticles,
5 GF-20 PPI-4 mm& 5 PPI-8 mm-Cu-0.01%
and alumina nanoparticles on the copper foam fibers can be
4.0x10
GF-20 PPI-4 mm& 5 PPI-8 mm-Cu-0.1% removed by diluted hydrochloric acid. The alumina density is
GF-20 PPI-4 mm& 5 PPI-8 mm-Cu-0.5%
3.98 g cm3. In the present study, the alumina nanoparticle
5
2.0x10 GF-20 PPI-4 mm& 5 PPI-8 mm-Cu
0.0
smooth copper plate
weights on GF-20 PPI–4 mm & 5 PPI–8 mm-Cu and GF-100 PPI–
0 10 20 30 40 4 mm & 5 PPI–8 mm-Cu are 0.08551 g and 0.3868 g, respectively.
ΔTsat(K)
Therefore, based on Eqs. (4) and (7), the mean thicknesses of
(a) 20 nm( 20 PPI=4 mm & 5 PPI=8 mm, Cu) deposited alumina nanoparticle on the two gradient foams are
0.85573 lm and 8.79834 lm, respectively. According to the fiber
6
diameter based on the microstructure model of metal foams [18],
1.4x10
the fiber radius of a foam layer is:
1.2x10
6
qffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
6
ri ¼ 0:0127 4ð1 ei Þ=ðp þ p2 Þ=xi ð8Þ
1.0x10
5 Based on Eq. (8), the fiber radius of the 100 PPI foam is 63 lm, the
8.0x10
q(W· m )
fiber radius of the 20 PPI foam is 315 lm, the fiber radius of the 5
-2
5
6.0x10 PPI foam is 1260 lm. The length of a foam layer is:
5 GF-20 PPI-4 mm& 5 PPI-8 mm-Cu-0.01%
qffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
4.0x10
GF-20 PPI-4 mm& 5 PPI-8 mm-Cu-0.1% li ¼ 0:0025 0:025 di xi 4ðp þ p2 Þ=ð1 ei Þ=ð2pr i 0:0254Þ
5
GF-20 PPI-4 mm& 5 PPI-8 mm-Cu-0.5%
2.0x10 GF-20 PPI-4 mm& 5 PPI-8 mm-Cu
ð9Þ
smooth copper plate
0.0
0 10 20 30 40 Then the average fiber radius of a gradient foam is:
ΔTsat(K)
rmean
(b) 50nm( Pn pffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
20 PPI=4 mm & 5 PPI=8 mm, Cu) ¼ 0:0025 0:025 di xi 4ðp þ p2 Þ=ð1 ei Þ=0:0254
i¼1
¼ Pn pffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffiffi
i¼1 ¼ 0:0025 0:025 di xi 4ðp þ p2 Þ=ð1 ei Þ=ð2pr i 0:0254Þ
1.4x10
6 ð10Þ
1.2x10
6 Based on Eq. (10), the average fiber radiuses of GF-20 PPI–4 mm
6
& 5 PPI–8 mm-Cu and GF-100 PPI–4 mm & 5 PPI–8 mm-Cu are
1.0x10
378.1 lm and 195.9 lm, respectively. Therefore, the fiber radius
8.0x10
5 incensement rates of GF-20 PPI–4 mm & 5 PPI–8 mm-Cu and GF-
q(W· m )
-2
5
100 PPI–4 mm & 5 PPI–8 mm-Cu are 0.226% and 4.49%, respective-
6.0x10 ly. Then the surface area incensement rate of GF-20 PPI–4 mm &
4.0x10
5
GF-20 PPI-4 mm& 5 PPI-8 mm-Cu-0.01% 5 PPI–8 mm-Cu is 0.226%, and GF-100 PPI–4 mm & 5 PPI–8 mm-
GF-20 PPI-4 mm& 5 PPI-8 mm-Cu-0.1%
GF-20 PPI-4 mm& 5 PPI-8 mm-Cu-0.5%
Cu is 4.49%. The results in Fig. 5(a) indicate that, in saturated
5
2.0x10 deionized water, pool boiling heat transfer the deposited gradient
GF-20 PPI-4 mm& 5 PPI-8 mm-Cu
smooth copper plate
0.0 foam GF-20 PPI–4 mm & 5 PPI–8 mm-Cu is remarkably lower than
0 10 20 30 40 that in 0.5% boiling alumina nanofluid due to the water’s lower
ΔTsat(K)
effective liquid thermal conductivity. Moreover, deposited alumina
(c) 100nm( 20 PPI=4 mm & 5 PPI=8 mm, Cu) nanoparticles decrease the effective thermal conductivity of cop-
per foam. Furthermore, SEM image shown in Fig. 5(c) reveals that
Fig. 4. Al2O3 nanoparticle concentration effect. deposited nanoparticles form the detached thin layer above the
fiber of gradient foam GF-20 PPI–4 mm & 5 PPI–8 mm-Cu, which
foams. The positive effect of the deposited alumina nanoparticles is significantly increases escaping resistance of the bubbles generat-
the surface area increment. However, alumina thermal conduc- ed on the fibers. Fig. 5(b) reveals that, in saturated deionized water,
tivity is far lower than the copper, which decreases the effective pool boiling heat transfer of the deposited gradient foam GF-
thermal conductivity of the gradient copper foam. Assuming that 100 PPI–4 mm & 5 PPI–8 mm-Cu is only slightly lower than that
metal foam fibers are cylindrical and their average radius is r and in 0.5% boiling alumina nanonfluid. SEM image in Fig. 5(d) shows
the nanoparticle layer thickness is d, the volume increment of a that, the layer sticks to the fiber surface of GF-100 PPI–4 mm &
gradient foam by nanoparticle layers is: 5 PPI–8 mm-Cu and deposited nanoparticles forms a lot of fissures
which can provide more nucleation sites. The positive effect of
X
n X
n
DV ¼ ½pðri þ dÞ l pr 2i l ¼
2 2
½2pr i dl þ pd l ð5Þ fissures partially offsets the negative effects of the lower liquid
i¼1 i¼1 conductivity of water and the downgrading copper foam effective
thermal conductivity by the deposited alumina nanoparticles.
When r i >> d, Eq. (5) can be simplified as:
X
n X
n 3.3. Surfactant effect
DV ¼ 2pr i dl ¼ Si d ¼ m=q ð6Þ
i¼1 i¼1
Fig. 6(a) indicates that, pool boiling heat transfer of GF-40 PPI–
Then the average nanoparticle thickness d on the foam fiber can 6 mm & 20 PPI–8 mm-Ni is heavily enhanced by 100 ppm SDS, and
be calculated as: the maximum boiling heat transfer coefficient increment is more
828 Z.G. Xu, C.Y. Zhao / International Journal of Heat and Mass Transfer 85 (2015) 824–829
6
1.4x10
6
1.2x10
6 1.0x10
6
1.0x10 5
8.0x10
5
8.0x10
q(W· m )
-2
q(W· m )
6.0x10
-2
5
6.0x10
5 5
4.0x10 4.0x10
GF-20 PPI-4 mm& 5 PPI-8 mm-Cu-0.01%
5 GF-40 PPI-6mm & 20 PPI-8 mm-Ni-100 ppm
2.0x10 GF-20 PPI-4 mm& 5 PPI-8 mm-Cu-after deposition
GF-40 PPI-6mm & 20 PPI-8 mm-Ni-400 ppm
GF-20 PPI-4 mm& 5 PPI-8mm-Cu 5
smooth copper plate
2.0x10 GF-40 PPI-6mm & 20 PPI-8 mm-Ni-800 ppm
0.0 GF-40 PPI-6mm & 20 PPI-8 mm-Ni
0 10 20 30 40 smooth copper plate
ΔTsat(K) 0.0
(a) 100nm Al2O3 nanoparticle deposition 0 10 20 30 40
ΔTsat(K)
(δ20 PPI=4 mm & δ5 PPI=8 mm, Cu)
1.4x10
6
(a) 40 PPI=6 mm & 20 PPI=8 mm, Ni
6
1.2x10
6
1.0x10 6
1.0x10 CHF
5
8.0x10
q(W· m )
-2
5
6.0x10
5 8.0x10
5 CHF
4.0x10 5
q(W· m )
6.0x10
GF-100 PPI-4 mm& 5 PPI-8 mm-0.5% -2
5 GF-100 PPI-4 mm& 5 PPI-8 mm-after deposition
2.0x10
GF-100 PPI-4 mm& 5 PPI-8mm
5
0.0
smooth copper plate 4.0x10
0 10 20 30 40 GF-100PPI-6mm & 5PPI-8mm-Ni-100ppm
ΔTsat(K) 5
GF-100PPI-6mm & 5PPI-8mm-Ni-400ppm
2.0x10 GF-100PPI-6mm & 5PPI-8mm-Ni-800ppm
(b) 100nm Al2O3 nanoparticle deposition GF-100PPI-6mm & 5PPI-8mm-Ni
(δ100 PPI=4 mm & δ5 PPI=8 mm, Cu) smooth copper plate
0.0
0 10 20 30 40
ΔTsat(K)
6
1.2x10
CHF
6
1.0x10
5
8.0x10
CHF
q(W· m )
-2
5
(c) SEM images after boing in 0.5vol% 100nm Al2O3 6.0x10
nanofluid (δ20 PPI=4 mm & δ5 PPI=8 mm, Cu)
5
4.0x10
GF-100PPI-6mm & 20PPI-6mm & 5PPI-8mm-100ppm
5 GF-100PPI-6mm & 20PPI-6mm & 5PPI-8mm-400ppm
2.0x10 GF-100PPI-6mm & 20PPI-6mm & 5PPI-8mm-800ppm
GF-100PPI-6mm & 20PPI-6mm & 5PPI-8mm
smooth copper plate
0.0
0 10 20 30 40
ΔTsat(K)
(d) SEM images after boing in 0.5vol% 100nm Al2O3 20 PPI–8 mm-Ni becomes deteriorated in the 800 ppm SDS solu-
nanofluid (δ100 PPI=4 mm & δ5 PPI=8 mm, Cu) tion. when the heat flux is over 9.2 105 W m2, pool boiling heat
transfer of GF-40 PPI-6 mm & 20 PPI–8 mm-Ni becomes deteriorat-
Fig. 5. Al2O3 nanoparticle deposition effect.
ed in the 400 ppm SDS solution. SDS seriously worsens the pool
boiling heat transfer of GF-100 PPI–6 mm & 5 PPI–8 mm-Ni, as
shown in Fig. 6(b). The connected pores of 100 PPI foam is very
than three times. However, pool boiling heat transfer enhancement small. When bubbles are escaping, the resistance suffering from
of GF-40 PPI–6 mm & 20 PPI–8 mm-Ni decreases with increasing foam skeleton will be very sensitive with the liquid viscosity incre-
SDS concentration because of the increasing liquid viscosity which ment. Based on the equation of Chu et al. [19], the expression for
prevents bubbles escaping. Even worse, when the heat flux is over CHF on a heated horizontal surface with microstructures can be
7 105 W m2, pool boiling heat transfer of GF-40 PPI–6 mm & obtained
Z.G. Xu, C.Y. Zhao / International Journal of Heat and Mass Transfer 85 (2015) 824–829 829
1=2
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